IndiumV3, Chine, Analysis, bibRecord, 000246

Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells

Identifieur interne : 000246 ( Chine/Analysis ); précédent : 000245; suivant : 000247

Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells

Auteurs : RBID : Pascal:13-0303887

Descripteurs français

Pascal (Inist)
- Point quantique, Cathode, Système tampon, Cellule solaire organique, Caractéristique électrique, Méthode hydrothermale, Synthèse hydrothermale, Additif, Niveau énergie, Couche ITO, Addition étain, Orbite, Etude comparative, Couche tampon, Conversion énergie, Taux conversion, Exciton, Recombinaison porteur charge, Polymère, Couche active, Graphène, Nanomatériau, Semiconducteur bande interdite large, Carbonate de césium, Oxyde d'indium, Ester, Acide butyrique, Composé du fullerène, Cs2CO3, ITO.
Wicri :
- concept : Polymère.

English descriptors

KwdEn :
- Active layer, Additive, Buffer layer, Buffer system, Butyric acid, Cathode, Cesium carbonate, Charge carrier recombination, Comparative study, Conversion rate, Electrical characteristic, Energy conversion, Energy level, Ester, Exciton, Fullerene compounds, Graphene, Hydrothermal growth, Hydrothermal synthesis, ITO layers, Indium oxide, Nanostructured materials, Orbit, Organic solar cells, Polymer, Quantum dot, Tin addition, Wide band gap semiconductors.

Abstract

Graphene quantum dots (GQDs) are an emerging class of nanomaterials with unique photonic and electric properties. In this study, GQDs were prepared by a facile, inexpensive and high-yield hydrothermal method and were further used as a cathode buffer additive for inverted polymer solar cells due to a wide band gap (∼3.3 eV) and well-matched energy level between GQDs-cesium carbonate (GQDs-Cs₂CO₃) modified indium tin oxide (3.8 eV) and high occupied molecular orbit of [6,6]-phenyl-C61-butyric acid methyl ester (3.7 eV). In comparison to inverted polymer solar cells using cesium carbonate (Cs₂CO₃) buffer layer, the power conversion efficiency of GQDs-Cs₂CO₃ based device showed 22% enhancement from 2.59% to 3.17% as a result of enhanced exciton dissociation and suppressed free charge recombination at cathode/polymer active layer interface by GQDs. This work provides a new application of GQDs in organic electronic devices.

Links toward previous steps (curation, corpus...)

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Links to Exploration step

Pascal:13-0303887

Le document en format XML

<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells</title>
<author><name>HONG BIN YANG</name>
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<s2>Singapore 637459</s2>
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<country>Singapour</country>
<wicri:noRegion>Singapore 637459</wicri:noRegion>
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</author>
<author><name>YONG QIAN DONG</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive</s1>
<s2>Singapore 637459</s2>
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</author>
<author><name>XIZU WANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Institute of Materials Research and Engineering, No. 3 Research Link</s1>
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<author><name>SI YUN KHOO</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive</s1>
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<author><name>BIN LIU</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive</s1>
<s2>Singapore 637459</s2>
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<author><name>CHANG MING LI</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive</s1>
<s2>Singapore 637459</s2>
<s3>SGP</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>4 aut.</sZ>
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<country>Singapour</country>
<wicri:noRegion>Singapore 637459</wicri:noRegion>
</affiliation>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Institute for Clean Energy & Advanced Materials, Southwest University</s1>
<s2>Chongqing 400715</s2>
<s3>CHN</s3>
<sZ>6 aut.</sZ>
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<country>République populaire de Chine</country>
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<date when="2013">2013</date>
<idno type="stanalyst">PASCAL 13-0303887 INIST</idno>
<idno type="RBID">Pascal:13-0303887</idno>
<idno type="wicri:Area/Main/Corpus">000748</idno>
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<seriesStmt><idno type="ISSN">0927-0248</idno>
<title level="j" type="abbreviated">Sol. energy mater. sol. cells</title>
<title level="j" type="main">Solar energy materials and solar cells</title>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Active layer</term>
<term>Additive</term>
<term>Buffer layer</term>
<term>Buffer system</term>
<term>Butyric acid</term>
<term>Cathode</term>
<term>Cesium carbonate</term>
<term>Charge carrier recombination</term>
<term>Comparative study</term>
<term>Conversion rate</term>
<term>Electrical characteristic</term>
<term>Energy conversion</term>
<term>Energy level</term>
<term>Ester</term>
<term>Exciton</term>
<term>Fullerene compounds</term>
<term>Graphene</term>
<term>Hydrothermal growth</term>
<term>Hydrothermal synthesis</term>
<term>ITO layers</term>
<term>Indium oxide</term>
<term>Nanostructured materials</term>
<term>Orbit</term>
<term>Organic solar cells</term>
<term>Polymer</term>
<term>Quantum dot</term>
<term>Tin addition</term>
<term>Wide band gap semiconductors</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Point quantique</term>
<term>Cathode</term>
<term>Système tampon</term>
<term>Cellule solaire organique</term>
<term>Caractéristique électrique</term>
<term>Méthode hydrothermale</term>
<term>Synthèse hydrothermale</term>
<term>Additif</term>
<term>Niveau énergie</term>
<term>Couche ITO</term>
<term>Addition étain</term>
<term>Orbite</term>
<term>Etude comparative</term>
<term>Couche tampon</term>
<term>Conversion énergie</term>
<term>Taux conversion</term>
<term>Exciton</term>
<term>Recombinaison porteur charge</term>
<term>Polymère</term>
<term>Couche active</term>
<term>Graphène</term>
<term>Nanomatériau</term>
<term>Semiconducteur bande interdite large</term>
<term>Carbonate de césium</term>
<term>Oxyde d'indium</term>
<term>Ester</term>
<term>Acide butyrique</term>
<term>Composé du fullerène</term>
<term>Cs2CO3</term>
<term>ITO</term>
</keywords>
<keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Polymère</term>
</keywords>
</textClass>
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<front><div type="abstract" xml:lang="en">Graphene quantum dots (GQDs) are an emerging class of nanomaterials with unique photonic and electric properties. In this study, GQDs were prepared by a facile, inexpensive and high-yield hydrothermal method and were further used as a cathode buffer additive for inverted polymer solar cells due to a wide band gap (∼3.3 eV) and well-matched energy level between GQDs-cesium carbonate (GQDs-Cs<sub>2</sub>
CO<sub>3</sub>
) modified indium tin oxide (3.8 eV) and high occupied molecular orbit of [6,6]-phenyl-C61-butyric acid methyl ester (3.7 eV). In comparison to inverted polymer solar cells using cesium carbonate (Cs<sub>2</sub>
CO<sub>3</sub>
) buffer layer, the power conversion efficiency of GQDs-Cs<sub>2</sub>
CO<sub>3</sub>
 based device showed 22% enhancement from 2.59% to 3.17% as a result of enhanced exciton dissociation and suppressed free charge recombination at cathode/polymer active layer interface by GQDs. This work provides a new application of GQDs in organic electronic devices.</div>
</front>
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<fA03 i2="1"><s0>Sol. energy mater. sol. cells</s0>
</fA03>
<fA05><s2>117</s2>
</fA05>
<fA08 i1="01" i2="1" l="ENG"><s1>Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>HONG BIN YANG</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>YONG QIAN DONG</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>XIZU WANG</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>SI YUN KHOO</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>BIN LIU</s1>
</fA11>
<fA11 i1="06" i2="1"><s1>CHANG MING LI</s1>
</fA11>
<fA14 i1="01"><s1>School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive</s1>
<s2>Singapore 637459</s2>
<s3>SGP</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Institute for Clean Energy & Advanced Materials, Southwest University</s1>
<s2>Chongqing 400715</s2>
<s3>CHN</s3>
<sZ>6 aut.</sZ>
</fA14>
<fA14 i1="03"><s1>Institute of Materials Research and Engineering, No. 3 Research Link</s1>
<s2>117602, Singapore</s2>
<s3>SGP</s3>
<sZ>3 aut.</sZ>
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<fA20><s1>214-218</s1>
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<fA21><s1>2013</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>18016</s2>
<s5>354000501971110350</s5>
</fA43>
<fA44><s0>0000</s0>
<s1>© 2013 INIST-CNRS. All rights reserved.</s1>
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<fA45><s0>27 ref.</s0>
</fA45>
<fA47 i1="01" i2="1"><s0>13-0303887</s0>
</fA47>
<fA60><s1>P</s1>
</fA60>
<fA61><s0>A</s0>
</fA61>
<fA64 i1="01" i2="1"><s0>Solar energy materials and solar cells</s0>
</fA64>
<fA66 i1="01"><s0>NLD</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Graphene quantum dots (GQDs) are an emerging class of nanomaterials with unique photonic and electric properties. In this study, GQDs were prepared by a facile, inexpensive and high-yield hydrothermal method and were further used as a cathode buffer additive for inverted polymer solar cells due to a wide band gap (∼3.3 eV) and well-matched energy level between GQDs-cesium carbonate (GQDs-Cs<sub>2</sub>
CO<sub>3</sub>
) modified indium tin oxide (3.8 eV) and high occupied molecular orbit of [6,6]-phenyl-C61-butyric acid methyl ester (3.7 eV). In comparison to inverted polymer solar cells using cesium carbonate (Cs<sub>2</sub>
CO<sub>3</sub>
) buffer layer, the power conversion efficiency of GQDs-Cs<sub>2</sub>
CO<sub>3</sub>
 based device showed 22% enhancement from 2.59% to 3.17% as a result of enhanced exciton dissociation and suppressed free charge recombination at cathode/polymer active layer interface by GQDs. This work provides a new application of GQDs in organic electronic devices.</s0>
</fC01>
<fC02 i1="01" i2="X"><s0>001D06C02D1</s0>
</fC02>
<fC02 i1="02" i2="X"><s0>230</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Point quantique</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Quantum dot</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Punto cuántico</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE"><s0>Cathode</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG"><s0>Cathode</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA"><s0>Cátodo</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE"><s0>Système tampon</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Buffer system</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Sistema amortiguador</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Cellule solaire organique</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Organic solar cells</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Caractéristique électrique</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Electrical characteristic</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA"><s0>Característica eléctrica</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Méthode hydrothermale</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Hydrothermal growth</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Método hidrotermal</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="3" l="FRE"><s0>Synthèse hydrothermale</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="3" l="ENG"><s0>Hydrothermal synthesis</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Additif</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Additive</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Aditivo</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Niveau énergie</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Energy level</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Nivel energía</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Couche ITO</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>ITO layers</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Addition étain</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Tin addition</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Adición estaño</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Orbite</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Orbit</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Orbita</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Etude comparative</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Comparative study</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Estudio comparativo</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Couche tampon</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Buffer layer</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Capa tampón</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="X" l="FRE"><s0>Conversion énergie</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="ENG"><s0>Energy conversion</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="SPA"><s0>Conversión energética</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Taux conversion</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Conversion rate</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Factor conversión</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Exciton</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Exciton</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Excitón</s0>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Recombinaison porteur charge</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Charge carrier recombination</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Recombinación portador carga</s0>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Polymère</s0>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Polymer</s0>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Polímero</s0>
<s5>19</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Couche active</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Active layer</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Capa activa</s0>
<s5>20</s5>
</fC03>
<fC03 i1="21" i2="X" l="FRE"><s0>Graphène</s0>
<s5>22</s5>
</fC03>
<fC03 i1="21" i2="X" l="ENG"><s0>Graphene</s0>
<s5>22</s5>
</fC03>
<fC03 i1="21" i2="X" l="SPA"><s0>Graphene</s0>
<s5>22</s5>
</fC03>
<fC03 i1="22" i2="3" l="FRE"><s0>Nanomatériau</s0>
<s5>23</s5>
</fC03>
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<s5>23</s5>
</fC03>
<fC03 i1="23" i2="3" l="FRE"><s0>Semiconducteur bande interdite large</s0>
<s5>24</s5>
</fC03>
<fC03 i1="23" i2="3" l="ENG"><s0>Wide band gap semiconductors</s0>
<s5>24</s5>
</fC03>
<fC03 i1="24" i2="X" l="FRE"><s0>Carbonate de césium</s0>
<s5>25</s5>
</fC03>
<fC03 i1="24" i2="X" l="ENG"><s0>Cesium carbonate</s0>
<s5>25</s5>
</fC03>
<fC03 i1="24" i2="X" l="SPA"><s0>Cesio carbonato</s0>
<s5>25</s5>
</fC03>
<fC03 i1="25" i2="X" l="FRE"><s0>Oxyde d'indium</s0>
<s5>26</s5>
</fC03>
<fC03 i1="25" i2="X" l="ENG"><s0>Indium oxide</s0>
<s5>26</s5>
</fC03>
<fC03 i1="25" i2="X" l="SPA"><s0>Indio óxido</s0>
<s5>26</s5>
</fC03>
<fC03 i1="26" i2="X" l="FRE"><s0>Ester</s0>
<s5>27</s5>
</fC03>
<fC03 i1="26" i2="X" l="ENG"><s0>Ester</s0>
<s5>27</s5>
</fC03>
<fC03 i1="26" i2="X" l="SPA"><s0>Ester</s0>
<s5>27</s5>
</fC03>
<fC03 i1="27" i2="X" l="FRE"><s0>Acide butyrique</s0>
<s2>NK</s2>
<s5>28</s5>
</fC03>
<fC03 i1="27" i2="X" l="ENG"><s0>Butyric acid</s0>
<s2>NK</s2>
<s5>28</s5>
</fC03>
<fC03 i1="27" i2="X" l="SPA"><s0>Butírico ácido</s0>
<s2>NK</s2>
<s5>28</s5>
</fC03>
<fC03 i1="28" i2="3" l="FRE"><s0>Composé du fullerène</s0>
<s5>29</s5>
</fC03>
<fC03 i1="28" i2="3" l="ENG"><s0>Fullerene compounds</s0>
<s5>29</s5>
</fC03>
<fC03 i1="29" i2="X" l="FRE"><s0>Cs2CO3</s0>
<s4>INC</s4>
<s5>82</s5>
</fC03>
<fC03 i1="30" i2="X" l="FRE"><s0>ITO</s0>
<s4>INC</s4>
<s5>83</s5>
</fC03>
<fN21><s1>287</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
</pA>
</standard>
</inist>
</record>

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   |texte=   Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells
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Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells

Graphene quantum dots-incorporated cathode buffer for improvement of inverted polymer solar cells

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